A unified stochastic formulation of dissipative quantum dynamics. II. Beyond linear response of spin baths
نویسندگان
چکیده
منابع مشابه
A unified stochastic formulation of dissipative quantum dynamics. II. Beyond linear response of spin baths.
We use the "generalized hierarchical equation of motion" proposed in Paper I [C.-Y. Hsieh and J. Cao, J. Chem. Phys. 148, 014103 (2018)] to study decoherence in a system coupled to a spin bath. The present methodology allows a systematic incorporation of higher-order anharmonic effects of the bath in dynamical calculations. We investigate the leading order corrections to the linear response app...
متن کاملA unified stochastic formulation of dissipative quantum dynamics. I. Generalized hierarchical equations.
We extend a standard stochastic theory to study open quantum systems coupled to a generic quantum environment. We exemplify the general framework by studying a two-level quantum system coupled bilinearly to the three fundamental classes of non-interacting particles: bosons, fermions, and spins. In this unified stochastic approach, the generalized stochastic Liouville equation (SLE) formally cap...
متن کاملDissipative quantum dynamics with the surrogate Hamiltonian approach. A comparison between spin and harmonic baths.
The dissipative quantum dynamics of an anharmonic oscillator coupled to a bath is studied with the purpose of elucidating the differences between the relaxation to a spin bath and to a harmonic bath. Converged results are obtained for the spin bath by the surrogate Hamiltonian approach. This method is based on constructing a system-bath Hamiltonian, with a finite but large number of spin bath m...
متن کاملQuantum Spin Dynamics (QSD) II
We continue here the analysis of the previous paper of the Wheeler-DeWitt constraint operator for four-dimensional, Lorentzian, non-perturbative, canonical vacuum quantum gravity in the continuum. In this paper we derive the complete kernel, as well as a physical inner product on it, for a non-symmetric version of the Wheeler-DeWitt operator. We then define a symmetric version of the Wheeler-De...
متن کاملDissipative Quantum Control of a Spin Chain.
A protocol is discussed for preparing a spin chain in a generic many-body state in the asymptotic limit of tailored nonunitary dynamics. The dynamics require the spectral resolution of the target state, optimized coherent pulses, engineered dissipation, and feedback. As an example, we discuss the preparation of an entangled antiferromagnetic state, and argue that the procedure can be applied to...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
ژورنال
عنوان ژورنال: The Journal of Chemical Physics
سال: 2018
ISSN: 0021-9606,1089-7690
DOI: 10.1063/1.5018726